Synthesis and Crystal Structure of the Octametallic Ferrocene Containing Molybdenum(V) Cluster Mo4(μ3-O)4(μ2-O2P(CH2)2Fc)4O4 and Crystal Structure of 1,1′-Bis(Chloromethyl)Ferrocene

Document Type

Article

Publication Date

9-2012

Department

Department of Chemistry

Abstract

The reaction of MoO 2(acac) 2 with 1,1′-[phosphinicobis(methylene)]-ferrocene in ethanol at 120 °C and in the presence of triethylamine results in the octametallic cluster Mo 4(μ 3-O) 4(μ 2-O 2P(CH 2) 2Fc) 4O 4. If the reaction is carried out in the absence of triethylamine a mixture of products are obtained of which the identity of the compound produced was hypothesized but not definitively established. Mo 4(μ 3-O) 4(μ 2-O 2P(CH 2) 2Fc) 4O 4 is characterized by IR and 31P-NMR spectroscopy along with the single crystal X-ray determination of its structure. The crystal structure of 1,1′-bis(chloromethyl)ferrocene is also detailed.

Publication Title

Journal of Cluster Science

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