Date of Award

2024

Document Type

Open Access Master's Report

Degree Name

Master of Science in Physics (MS)

Administrative Home Department

Department of Physics

Advisor 1

Yoke Khin Yap

Advisor 2

Jae Yong Suh

Committee Member 1

John Jaszczak

Abstract

Monolayers of transition metal dichalcogenides (TMDCs) have attracted significant attention as the rare two-dimensional (2D) semiconducting materials with a direct energy band gap. Chemical vapour deposition (CVD) is one of the scalable techniques to grow atomically thin TMDC monolayers in high quality, but it requires high growth temperature. Herein we report the growth of MoS2, WS2 and MoSe2 by a one-step halide-assisted CVD method using NaCl and KCl as the catalysts. These halides could reduce the growth temperature of TMDCS by reacting with the precursors (TMDC powders) to form volatile intermediate compounds as the growth species. We use optical microscopy, scanning electron microscopy (SEM) and atomic force microscopy (AFM) techniques to study the morphological properties of the CVD-grown TMDCs. We were subsequently successful to transfer the CVD-grown monolayers into desired target substrates using chemical etching method.

Available for download on Wednesday, July 16, 2025

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