First-principles study of the structural, electronic, and optical properties of Ga2 O3 in its monoclinic and hexagonal phases

Document Type

Article

Publication Date

12-5-2006

Abstract

We report the results of a comprehensive study on the structural, electronic, and optical properties of Ga2 O3 in its ambient, monoclinic (β) and high-pressure, hexagonal (α) phases in the framework of all-electron density functional theory. In both phases, the conduction band minimum is at the zone center while the valance band maximum is rather flat in the k space. The calculated electron effective mass me* m0 comes out to be 0.342 and 0.276 for β- Ga2 O3 and α- Ga2 O3, respectively. The dynamic dielectric function, reflectance, and energy-loss function for both phases are reported for a wide energy range of 0-50 eV. The subtle differences in electronic and optical properties can be attributed to the higher symmetry, coordination number of Ga atoms, and packing density in α- Ga2 O3 relative to that in β- Ga2 O3. © 2006 The American Physical Society.

Publication Title

Physical Review B - Condensed Matter and Materials Physics

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